Gold Catalysis: No Steric Limitations in the Phenol Synthesis

D. Hackenberger, L. Huang, L. J. Gooßen15th Belgian Organic Synthesis Symposium 2016, Antwerp

Gold catalysis for organic synthesis.

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Gold catalysis for organic synthesis

Light-mediated photoredox transformations have become commonplace in contemporary catalysis research and design. Excited-state redox catalysts trigger photoinduced electron transfers (PET) through oxidative or reductive quenching modes, allowing access to one-electron variations of classic radical reactions and the discovery of new transformations in organic chemistry. Herein, the use of Au-based photoredox catalysts containing powerful redox properties along with the emergence of dual catalyzed organic transformations involving photoredox catalysis and Au complexes for the Au(I)/Au(III) redox couple without use of stoichiometric oxidants will be discussed.1 Principles of Photochemistry and Gold2 Photoredox Transformations with Dimeric Gold Complexes3 Dual Catalysis Involving Au(I)/Au(III) Redox Cycles4 Concluding Remarks

A. Biafora, L. Huang, G. Zhang, V. Bragoni, L. J. Gooßen15th Belgian Organic Synthesis Symposium 2016, Antwerp

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19/07/2011 · Gold-catalyzed oxidation in organic synthesis: a promise kept ..


Practical Catalysis - Streamlined Organic Synthesis

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Synthesis & Catalysis | imedpub | journal

The past decade has witnessed a remarkable growth in the number of organic reactions that are catalyzed by homogeneous gold complexes. Many of the early reported reactions took advantage of the propensity of gold complexes to serve as excellent catalysts for reactions that proceed through π-activation of carbon–carbon multiple bonds. Subsequently, the reactivity paradigms available for gold complexes have proven to be almost limitless. The contributions from over 25 research groups from 13 countries underscore the growing importance of homogenous gold catalysis. More importantly, the papers in this Thematic Series highlight the remarkable breath of reactivity that can be accessed using homogenous gold complexes as catalysts; from catalysis of sigmatropic rearrangement, cycloaddition and cycloisomerization reactions, to applications in enantioselective catalysis, oxidative coupling and the total synthesis of natural products, and transformations of alkynes, allenes, alkenes and even C–H bonds. A true treasure chest of reactivity!